Almost for sure initial ranging was done by radar. As radar became more advanced following WW2, the Moon loomed large in the sky as a giant target, who could resist?
In 1946 a modified military radar signal at 111.5 MHz was successfully bounced off the Moon and received. The following is from K3PGP's Experimenter's.Corner post Radar Echoes From the Moon January 1946 by Jack Mofenson, Evans Signal Laboratory, Belmar N.J.
THE RECENT EXPERIMENTS performed by the Signal Corps Engineering Laboratories in receiving radar echoes from the moon have aroused much comment from engineers, astronomers and others engaged in technical pursuits. Although the scientific aspects of sending radio frequency signals through the ionosphere are certainly of importance, the work done on the project is better classified as an engineering achievement. As yet, no long term systematic observations have been made. This article is confined, therefore, to a discussion of the technical characteristics and general description of the equipment employed.
Briefly, the experiment consisted of transmitting quarter second pulses of radio frequency energy at 111.5 mc every four seconds in the direction of the moon, and detecting echo signals approximately 2.5 seconds after transmission. Display of the detected signals was audible as well as visible. Technically, the experiment utilized well established radar techniques, but with radically different constants throughout the system. Considerations of pulse width, receiver bandwidth, transmitter power and the precise frequency of the returned signal due to Doppler effect, were such that careful attention had to be given to the design of the overall equipment.
After preliminary calculations were made concerning transmitter power, the reflectivity coefficient of the target, and receiver noise figure, it was apparent that receiving radar echoes from the moon was technically possible. Under the direction of Lt. Col. John H. DeWitt, a project called "project Diana" was set up in September 1945 to develop a radar system capable of transmitting rf pulses to the moon, and detecting echoes more than 2 seconds later. Prior to entering the Signal Corps, Colonel DeWitt, who at that time was chief engineer of Radio Station WSM in Nashville, Tenn., designed and constructed transmitting and receiving equipment for the purpose of receiving echoes from the moon. This equipment employed substantially similar transmitter power and frequency to that used by the Signal Corps, but the attempt was a failure due to insufficient sensitivity in the receiver. Colonel DeWitt's appreciation of the problem and personal supervision were the driving forces that made the present experiment successful. Assisting Lt. Colonel DeWitt were: E. K. Stodola, Dr. Harold D. Webb, Herbert P. Kauffman and the writer, all of Evans Signal Laboratory. Credit is also due the members of the Antenna and Mechanical Design Croup, Research Section, Theoretical Studies Group and others.
The practical implications of radar contact with the moon are numerous. During the war the Germans used the V2 Rocket which climbed some 70 miles above the earth, and the future holds the unhappy prospect of missiles going far higher than this. The matter of transmission of radio signals to great distances above the earth for detection and control of such weapons becomes a problem of military importance. Further, the use of a reflector far beyond the earth for radio waves makes possible direct measurement of the ability of radio waves to penetrate the ionosphere. A more complete investigation in this direction is indicated. The possibility of using the moon as the reflector for a part time long distance point to point communication system is also being considered, as well as using the moon as a target to measure field strength patterns.
By 1965 radar ranging measurements and topography mapping of the Moon had become fairly accurate. According to the 1965 IAU Symposium contribution The mean distance to the Moon as determined by radar all of the other errors had been managed and the limits on the absolute range (a few hundred meters) was the propagation velocity!
It seems that the speed of radio waves in a vacuum was uncertain to about 1 part per million in 1965. Certainly by the time that nanosecond lasers were starting to make ranging measurements, the errors on the radar ranging would have been sufficiently reduced to make them comparable with the requirements for time-gating of the protonic measurements.
Distance measurements point-to-point were not the limiting factors here though. The uncertainty in the diameter of the Moon itself made the final determination of the separation of body centers uncertain to 1.1 kilometer!
Recent geodetic determination of the Earth’s equatorial radius (Kuala 4, Fischer 5) indicate that a correction of about -100 m to the value of a given in table I is required. Hence, with Δr=-0.1 km and allowing for an error of Δb = ±1km, and Δc = ±300m, the final result becomes
$\bar{s}$=384400.2 km ±1.1km.
The accuracy of the value of $\bar{s} in the radar method is limited primarily by the uncertainties of the lunar radius and the velocity of radio wave propagation.